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Linking renewables and fossil fuels with carbon capture via energy storage for a sustainable energy future

Dawid P. Hanak, Vasilije Manovic

《化学科学与工程前沿（英文）》 2020年第14卷第3期页码 453-459 doi: 10.1007/s11705-019-1892-2

摘要： Renewable energy sources and low-carbon power generation systems with carbon capture and storage (CCS) are expected to be key contributors towards the decarbonisation of the energy sector and to ensure sustainable energy supply in the future. However, the variable nature of wind and solar power generation systems may affect the operation of the electricity system grid. Deployment of energy storage is expected to increase grid stability and renewable energy utilisation. The power sector of the future, therefore, needs to seek a synergy between renewable energy sources and low-carbon fossil fuel power generation. This can be achieved via wide deployment of CCS linked with energy storage. Interestingly, recent progress in both the CCS and energy storage fields reveals that technologies such as calcium looping are technically viable and promising options in both cases. Novel integrated systems can be achieved by integrating these applications into CCS with inherent energy storage capacity, as well as linking other CCS technologies with renewable energy sources via energy storage technologies, which will maximise the profit from electricity production, mitigate efficiency and economic penalties related to CCS, and improve renewable energy utilisation.

关键词： carbon capture energy storage renewable energy sources decarbonisation fossil fuels

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Biofuels and food security

Dmitry S. STREBKOV

《农业科学与工程前沿（英文）》 2015年第2卷第1期页码 1-12 doi: 10.15302/J-FASE-2015052

摘要： The major source of energy comes from fossil fuels. The current situation in the field of fuel and energy is becoming more problematic as world population continues to grow because of the limitation of fossil fuels reserve and its pressure on environment. This review aims to find economic, reliable, renewable and non-polluting energy sources to reduce high energy tariffs in Russian Federation. Biofuel is fuel derived directly from plants, or indirectly from agricultural, commercial, domestic, and/or industrial wastes. Other alternative energy sources including solar energy and electric power generation are also discussed. Over 100 Mt of biomass available for energy purposes is produced every year in Russian. One of the downsides of biomass energy is its potential threatens to food security and forage industries. An innovative approach proved that multicomponent fuel (80% diesel oil content for motor and 64% for in stove fuel) can remarkably reduce the costs. This paper proposed that the most promising energy model for future is based on direct solar energy conversion and transcontinental terawatt power transmission with the use of resonant wave-guide technology.

关键词： fossil fuels biofuels food security electric power solar energy

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The energy-environment nexus: aerosol science and technology enabling solutions

Pratim BISWAS, Wei-Ning WANG, Woo-Jin AN

《环境科学与工程前沿（英文）》 2011年第5卷第3期页码 299-312 doi: 10.1007/s11783-011-0351-1

摘要： Energy issues are important and consumption is slated to increase across the globe in the future. The energy-environment nexus is very important as strategies to meet future energy demand are developed. To ensure sustainable growth and development, it is essential that energy production is environmentally benign. There are two temporal issues—one that is immediate, and needs to address the environmental compliance of energy generation from fossil fuel sources; and second that is the need to develop newer alternate and more sustainable approaches in the future. Aerosol science and technology is an enabling discipline that addresses the energy issue over both these time scales. The paper is a review of aspects of aerosol science and engineering that helps address carbon neutrality of fossil fuels. Advanced materials to meet these challenges are discussed. Future approaches to effective harvesting of sunlight that are enabled by aerosol studies are discussed.

关键词： energy-environment nexus aerosol science and technology fossil fuels carbon dioxide conversion solar energy nanoparticle technology

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Production of hydrogen from fossil fuel: A review

《能源前沿（英文）》 2023年第17卷第5期页码 585-610 doi: 10.1007/s11708-023-0886-4

摘要： Production of hydrogen, one of the most promising alternative clean fuels, through catalytic conversion from fossil fuel is the most technically and economically feasible technology. Catalytic conversion of natural gas into hydrogen and carbon is thermodynamically favorable under atmospheric conditions. However, using noble metals as a catalyst is costly for hydrogen production, thus mandating non-noble metal-based catalysts such as Ni, Co, and Cu-based alloys. This paper reviews the various hydrogen production methods from fossil fuels through pyrolysis, partial oxidation, autothermal, and steam reforming, emphasizing the catalytic production of hydrogen via steam reforming of methane. The multicomponent catalysts composed of several non-noble materials have been summarized. Of the Ni, Co, and Cu-based catalysts investigated in the literature, Ni/Al₂O₃ catalyst is the most economical and performs best because it suppresses the coke formation on the catalyst. To avoid carbon emission, this method of hydrogen production from methane should be integrated with carbon capture, utilization, and storage (CCUS). Carbon capture can be accomplished by absorption, adsorption, and membrane separation processes. The remaining challenges, prospects, and future research and development directions are described.

关键词： methane catalytic conversion natural gas hydrogen production CCUS

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Evaluation of renewable energies production potential in the Middle East: confronting the world’s energy crisis

Hamid BAHRAMPOUR, Amir Khosro BEHESHTI MARNANI, Mohammad Bagher ASKARI, Mohammad Reza BAHRAMPOUR

《能源前沿（英文）》 2020年第14卷第1期页码 42-56 doi: 10.1007/s11708-017-0486-2

摘要： Oil and fossil fuels, the main source of energy in the Middle East have obviously the most destructive effects on the environment and public health. The developed countries of the Middle East are faced with the crisis and energy security. This paper is about evaluating the energy demand /consumption in the Middle East. First, the position of energy consumption in the world and the Middle East is discussed. Next, the evaluation of the current potential of clean energy production from renewable energies is explained. Finally, according to related maps, charts and information presented for the condition of renewable energy which has been approved by the countries of the Middle East, the greatest places in some countries of this region are introduced and discussed.

关键词： Middle East countries renewable energy fossil fuels energy crisis

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Review on design, preparation and performance characterization of gelled fuels for advanced propulsion

《化学科学与工程前沿（英文）》 2022年第16卷第6期页码 819-837 doi: 10.1007/s11705-021-2122-2

摘要： With the increasing demand for high-performance and safe fuels in aerospace propulsion systems, gelled fuels have attracted increasing attention. Because of their unique structure, gelled fuels exhibit the advantages of both solid and liquid fuels, such as high energy density, controllable thrust and storage safety. This review provides an overview on design, preparation and performance characterization of gelled fuels. The composition, preparation process and gelation mechanism of gelled high-energy-density fuels are described. Considering these aspects, the rheology and flow behavior of gelled fuels is summarized in terms of the shear thinning property, dynamic viscoelasticity and thixotropy. Moreover, the progress of atomization of gelled fuels is reviewed with a focus on the effect of atomizing nozzles. In addition, the experiments and theoretical models of single droplet combustion and combustor combustion are described. Finally, research directions for the development and application of gelled fuels are suggested.

关键词： gelled fuels high-energy-density fuels rheological properties atomization combustion

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Oxidative desulfurization of fuels using ionic liquids: A review? ?

Hua Zhao,Gary A. Baker

《化学科学与工程前沿（英文）》 2015年第9卷第3期页码 262-279 doi: 10.1007/s11705-015-1528-0

摘要： Extractive oxidation, wherein aromatic sulfur-containing compounds are extracted and subsequently oxidized to their corresponding sulfones, has proven to be one of the most effective desulfurization methods for producing ultra-low sulfur content fuels. As non-volatile and highly designable solvents, ionic liquids (ILs) have attracted considerable attention for the oxidative desulfurization of fuels. In this review, we systematically discuss the utility of ILs in catalytic and extractive oxidation, including their role as extractant, catalyst, or both. We also discuss the challenges facing the use of ILs in this regard, including their relatively high cost and excessive viscosity, as well as their efficiency and stability as catalyst.

关键词： oxidative desulfurization ionic liquids extraction fuels petroleum polyoxometalates

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Catalytic cracking of endothermic fuels in coated tube reactor

LI Jia, ZOU Jijun, ZHANG Xiangwen, GUO Wei, MI Zhentao

《化学科学与工程前沿（英文）》 2008年第2卷第2期页码 181-185 doi: 10.1007/s11705-008-0032-1

摘要： Suspensoid of HZSM-5 or HY zeolites mixed with a self-made ceramic-like binder was coated on the inner wall of a tubular reactor by gas-aided fluid displacement technology. The coated zeolites were characterized by means of X-ray diffraction (XRD), Fourier transform infrared spectroscopy (FT-IR) and scanning electron microscopy (SEM). The coating thickness is 10–20 ?m and the particle size of the zeolites is in the range of 1–5 ?m. In the coated reactor, cracking of endothermic fuels including -dodecane and aviation fuel RP-3 was carried out separately under supercritical conditions at 600°C and 625°C to investigate their heat sinks and conversion of catalytic reactions. For the reaction catalyzed by HY(25% mass fraction) coating, the heat sink capacity of -dodecane are 815.7 and 901.9 kJ/kg higher than that of the bare tube at 600°C and at 625°C, respectively. Conversion of -dodecane also increases from 42% to 60% at 600°C and from 66% to 80% at 625°C. The coated zeolite can significantly inhibit the carbon deposition during supercritical cracking reactions.

关键词： HZSM-5 self-made ceramic-like gas-aided Conversion Suspensoid

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Deep desulfurization of diesel fuels by catalytic oxidation

YU Guoxian, CHEN Hui, LU Shanxiang, ZHU Zhongnan

《化学科学与工程前沿（英文）》 2007年第1卷第2期页码 162-166 doi: 10.1007/s11705-007-0030-8

摘要： Reaction feed was prepared by dissolving dibenzothiophene (DBT), which was selected as a model organosulfur compound in diesel fuels, in -octane. The oxidant was a 30 wt-% aqueous solution of hydrogen peroxide. Catalytic performance of the activated carbons with saturation adsorption of DBT was investigated in the presence of formic acid. In addition, the effects of activated carbon dosage, formic acid concentration, initial concentration of hydrogen peroxide, initial concentration of DBT and reaction temperature on the oxidation of DBT were investigated. Experimental results indicated that performic acid and the hydroxyl radicals produced are coupled to oxidize DBT with a conversion ratio of 100%. Catalytic performance of the combination of activated carbon and formic acid is higher than that of only formic acid. The concentration of formic acid, activated carbon dosage, initial concentration of hydrogen peroxide and reaction temperature affect the oxidative removal of DBT. The higher the initial concentration of DBT in the -octane solution, the more difficult the deep desulfurization by oxidation is.

关键词： organosulfur compound performic presence activated hydrogen peroxide

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Extractive desulfurization of model fuels with a nitrogen-containing heterocyclic ionic liquid

《化学科学与工程前沿（英文）》 2022年第16卷第12期页码 1735-1742 doi: 10.1007/s11705-022-2167-x

摘要： A nitrogen-containing ionic liquid was synthesized using an aromatic nitrogen-containing heterocyclic and an amino acid, and applied to the extractive desulfurization process to remove benzothiophene, dibenzothiophene, and 4,6-dimethyldibenzothiphene from a model fuel oil. Chemical characterizations and simulation using Gaussian 09 software confirmed the rationality of an ionic liquid structure. Classification of non-covalent interactions between the ionic liquid and the three sulfur-containing contaminants was studied by reduced density gradient analysis. The viscosity of the ionic liquid was adjusted by addition of polyethylene glycol. Under extraction conditions of the volume of ionic liquid to oil as 1:1 and temperature as room temperature, the desulfurization selectivity of ionic liquid followed the order of 4,6-dimethyldibenzothiphene (15 min) < benzothiophene (15 min) ≈ dibenzothiophene (10 min). Addition of p-xylene and cyclohexene to the fuel oil had little effect. The extractant remained stable and effective after multiple regeneration cycles.

关键词： extractive desulfurization nitrogen-containing heterocyclic ionic liquid reduced density gradient analysis desulfurization selectivity

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A comparative study of particle size distribution from two oxygenated fuels and diesel fuel

Xiaoyan SHI, Kebin HE, Jie ZHANG, Yongliang MA, Yunshan GE, Jianwei TAN,

《环境科学与工程前沿（英文）》 2010年第4卷第1期页码 30-34 doi: 10.1007/s11783-010-0011-x

摘要： Oxygenated fuels are known to reduce particulate matter (PM) emissions from diesel engines. In this study, 100% soy methyl ester (SME) biodiesel fuel (B100) and a blend of 10% acetal denoted by A-diesel with diesel fuel were tested as oxygenated fuels. Particle size and number distributions from a diesel engine fueled with oxygenated fuels and base diesel fuel were measured using an Electrical Low Pressure Impactor (ELPI). Measurements were made at ten steady-state operational modes of various loads at two engine speeds. It was found that the geometric mean diameters of particles from SME and A-diesel were lower than that from base diesel fuel. Compared to diesel fuel, SME emitted more ultra-fine particles at rated speed while emitting less ultra-fine particles at maximum speed. Ultra-fine particle number concentrations of A-diesel were much higher than those of base diesel fuel at most test modes.

关键词： oxygenated fuel diesel particulate matter particle size distribution biofuel

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Production of renewable fuels by blending bio-oil with alcohols and upgrading under supercritical conditions

Sainab Omar, Suzanne Alsamaq, Yang Yang, Jiawei Wang

《化学科学与工程前沿（英文）》 2019年第13卷第4期页码 702-717 doi: 10.1007/s11705-019-1861-9

摘要： The work studied a non-catalytic upgrading of fast pyrolysis bio-oil by blending under supercritical conditions using methanol, ethanol and isopropanol as solvent and hydrogen donor. Characterisation of the bio-oil and the upgraded bio-oils was carried out including moisture content, elemental content, pH, heating value, gas chromatography-mass spectrometry (GCMS), Fourier transform infrared radiation, C nuclear magnetic resonance spectroscopy, and thermogravimetric analysis to evaluate the effects of blending and supercritical reactions. The GCMS analysis indicated that the supercritical methanol reaction removed the acids in the bio-oil consequently the pH increased from 2.39 in the crude bio-oil to 4.04 after the supercritical methanol reaction. The ester contents increased by 87.49% after the supercritical methanol reaction indicating ester formation could be the major deacidification mechanism for reducing the acidity of the bio-oil and improving its pH value. Simply blending crude bio-oil with isopropanol was effective in increasing the C and H content, reducing the O content and increasing the heating value to 27.55 from 17.51 MJ·kg in the crude bio-oil. After the supercritical isopropanol reaction, the heating value of the liquid product slightly further increased to 28.85 MJ·kg .

关键词： bio-oil blending supercritical upgrading characterisation

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火力发电厂绿色设计的研究

戴洪军,郭纪中,成虎

《中国工程科学》 2009年第11卷第9期页码 59-63

摘要：

火力发电厂资源消耗和污染物排放水平的高低，不仅关系到项目本身的生存与发展，而且影响到整个行业节能减排的实施，维系着全国经济和社会发展总体目标的实现。随着可持续发展理念的不断深入，绿色建筑技术和绿色设计技术已越来越广泛地被采纳和运用。通过在火电厂方案设计过程中开展绿色设计工作，采用模块化组合设计，优化设备及功能子系统，选用新技术、新工艺和新材料，采取有效的节水措施，实施控制系统优化方案，不但可以实现火电厂自身的可持续发展，而且能够取得良好的经济、社会和环境效益。通过初步研究，旨在为火电厂的绿色设计提供一些有益的经验积累。

关键词：可持续发展火力发电厂绿色设计绿色建筑节能减排

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Life cycle analysis and choice of natural gas-based automotive alternative fuels in Chongqing Municipality

WU Rui, LI Guangyi, ZHANG Zongyi, REN Yulong, HAN Weijian

《环境科学与工程前沿（英文）》 2007年第1卷第3期页码 292-298 doi: 10.1007/s11783-007-0049-6

摘要： Road transport produces significant amounts of emissions by using crude oil as the primary energy source. A reduction of emissions can be achieved by implementing alternative fuel chains. The objective of this study is to carry out an economic, environmental and energy (EEE) life cycle study on natural gas-based automotive fuels with conventional gasoline in an abundant region of China. A set of indices of four fuels/vehicle systems on the basis of life cycle are assessed in terms of impact of EEE, in which natural gas produces compressed natural gas (CNG), methanol, dimethylether (DME) and Fischer Tropsch diesel (FTD). The study included fuel production, vehicle production, vehicle operation, infrastructure and vehicle end of life as a system for each fuel/vehicle system. A generic gasoline fueled car is used as a baseline. Data have been reviewed and modified based on the best knowledge available to Chongqing local sources. Results indicated that when we could not change electric and hydrogen fuel cell vehicles into commercial vehicles on a large scale, direct use of CNG in a dedicated or bi-fuel vehicle is an economical choice for the region which is most energy efficient and more environmental friendly. The study can be used to support decisions on how natural gas resources can best be utilized as a fuel/energy resource for automobiles, and what issues need to be resolved in Chongqing. The models and approaches for this study can be applied to other regions of China as long as all the assumptions are well defined and modified to find a substitute automotive energy source and establish an energy policy in a specific region.

关键词： dedicated primary economic alternative abundant

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减排二氧化碳发展低碳经济首先要重视节约使用化石能源

曹湘洪

《中国工程科学》 2010年第12卷第8期页码 8-21

摘要：

分析了能源消费和经济发展的规律，可再生能源的特点、大量开发利用存在的技术瓶颈和减排二氧化碳的效果，认为我国能源消费总量正处在持续增长期，未来40年内可再生能源不可能成为我国的主要能源，化石能源仍将是我国能源的主体，提出减排二氧化碳、发展低碳经济，要首先重视节约使用化石能源。归纳了我国化石能源开发利用取得的成就和存在的问题，提出了节约使用化石能源的对策，一是确定比较合理的GDP增长速度，建立化石能源消费总量控制指标体系；二是建立化石能源加工利用过程全寿命周期能效及二氧化碳排放的评价方法，通过不断优化提高化石能源利用效率；三是从我国化石能源资源状况出发，研究建立符合国情的低碳现代化生活消费模式；四是充分利用财政税收政策和行政手段鼓励和强制节能；五是加强节约使用化石能源的技术、材料、产品的研究开发和推广应用；六是加大资金投入，实现化石能源的优化利用和节约使用。

关键词：二氧化碳低碳经济化石能源